"Persistent spin excitations in doped antiferromagnets revealed by resonant inelastic light scattering"

C. J. Jia: E. A. Nowadnick, K. Wohlfeld, Y. F. Kung, C.-C. Chen, S. Johnston, T. Tohyama, B. Moritz & T. P. Devereaux; Nature Communications, 02/28/14.

Additional Authors: E. A. Nowadnick, K. Wohlfeld, Y. F. Kung, C.-C. Chen, S. Johnston, T. Tohyama, B. Moritz & T. P. Devereaux

Abstract:

How coherent quasiparticles emerge by doping quantum antiferromagnets is a key question in correlated electron systems, whose resolution is needed to elucidate the phase diagram of copper oxides. Recent resonant inelastic X-ray scattering (RIXS) experiments in hole-doped cuprates have purported to measure high-energy collective spin excitations that persist well into the overdoped regime and bear a striking resemblance to those found in the parent compound, challenging the perception that spin excitations should weaken with doping and have a diminishing effect on superconductivity. Here we show that RIXS at the Cu L3-edge indeed provides access to the spin dynamical structure factor once one considers the full influence of light polarization. Further we demonstrate that high-energy spin excitations do not correlate with the doping dependence of Tc, while low-energy excitations depend sensitively on doping and show ferromagnetic correlations. This suggests that high-energy spin excitations are marginal to pairing in cuprate superconductors.